Nitrate-dominant visibility degradation during haze events in urban Beijing: A seasonal study on light extinction by second PMF method.
编号:1362
稿件编号:322 访问权限:仅限参会人
更新:2021-06-15 21:30:53 浏览:757次
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摘要
A transition to nitrate-dominant in aerosol chemical composition have been observed in recent years. However, detailed knowledge on the relationships between the changed aerosol components and light extinction is less known. Here a second PMF (PMF2) method was introduced to explore light extinction apportionment. The result showed that nitrate ammonium (AN) was the dominant factors to light extinction in all seasons, and its contribution increased with aerosol mass loadings, highlighting the critical role of nitrate in both mass concentration and light extinction. Secondary organic aerosols (SOA) were also important factors, but showed higher contribution under relatively clean periods. We also explore the changes of light extinction after COVID-19 breakout. Extinction coefficient (bext) increased by 18-72%, which was mainly caused by AN and SOA. Considering enhanced contribution and high hygroscopicity of nitrate, our result highlight the significance of a strict emission control of nitrogen oxides (NOx) and ammonia (NH3).
关键字
light extinction, nitrate ammonium, Beijing
稿件作者
李智杰
中国科学院大气物理研究所
孙业乐
中国科学院大气物理研究所
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